They Cage the Animals at Night. To this day it’s the only non-fiction book I read, and even though it was for a school class, I really enjoyed it and glad I read it as I never would have taken it off a bookshelf otherwise. Very powerful and emotional story.
I’ve never spent all my money on one series, but the first I got all the books for myself (not as gifts or through my parents when I was a kid) was Full Metal Alchemist. For more traditional books it would have been Spice & Wolf.